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Journal Articles

A Science-based mixed oxide property model for developing advanced oxide nuclear fuels

Kato, Masato; Oki, Takumi; Watanabe, Masashi; Hirooka, Shun; Vauchy, R.; Ozawa, Takayuki; Uwaba, Tomoyuki; Ikusawa, Yoshihisa; Nakamura, Hiroki; Machida, Masahiko

Journal of the American Ceramic Society, 107(5), p.2998 - 3011, 2024/05

 Times Cited Count:0 Percentile:0.01(Materials Science, Ceramics)

JAEA Reports

Survey and proposal for Japanese-English bilingual translation of technical terms focusing on nuclear disaster prevention

Togawa, Orihiko; Okuno, Hiroshi

JAEA-Review 2023-043, 94 Pages, 2024/03

JAEA-Review-2023-043.pdf:1.53MB

In order to translate nuclear disaster prevention documents written in Japanese into English, the Basic Act on Disaster Management, the Act on Special Measures Concerning Nuclear Emergency Preparedness, and the Convention on Nuclear Safety were surveyed for corresponding terms in Japanese and English. The survey results were integrated and unified English translations were selected. As a result, a Japanese-English correspondence table of technical terms in the field of nuclear disaster prevention was prepared and proposed.

Journal Articles

Nuclear data as foundation of nuclear research and development

Fukahori, Tokio; Nakayama, Shinsuke; Katabuchi, Tatsuya*; Shigyo, Nobuhiro*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 65(12), p.726 - 727, 2023/12

The Investigative Committee on Nuclear Data investigates and observes global trends in nuclear research and development and conducts comprehensive examinations of Japanese nuclear data activities from a broader perspective, as well as cooperation with domestic and foreign academic institutions in a wide range of fields other than the Atomic Energy Society. We aim to establish a system for communication, information exchange, and interdisciplinary cooperation. In this report, we will report on three of the main activities for the 2021-2022 term: a request list site for nuclear data, human resource development, and roadmap production.

JAEA Reports

Study of fabrication of SiC-matrixed fuel compact for HTGR

Kawano, Takahiro*; Mizuta, Naoki; Ueta, Shohei; Tachibana, Yukio; Yoshida, Katsumi*

JAEA-Technology 2023-014, 37 Pages, 2023/08

JAEA-Technology-2023-014.pdf:2.35MB

Fuel compact for High Temperature Gas-cooled Reactor (HTGR) is fabricated by calcinating a matrix consisting of graphite and binder with the coated fuel particle. The SiC-matrixed fuel compact uses a new matrix made of silicon carbide (SiC) replacing the conventional graphite. Applying the SiC-matrixed fuel compact for HTGRs is expected to improve their performance such as power densities. In this study, the sintering conditions for applying SiC as the matrix of fuel compacts for HTGR are selected, and the density and thermal conductivity of the prototype SiC are measured.

Journal Articles

Investigation of potential of vacuum-free femtosecond laser sintering for direct printing using silicon carbide nanoparticles without inorganic binder

Kawabori, Tatsuru*; Watanabe, Masashi; Imai, Yoshiyuki; Ueta, Shohei; Yan, X.; Mizoshiri, Mizue*

Applied Physics A, 129(7), p.498_1 - 498_9, 2023/07

 Times Cited Count:0 Percentile:0(Materials Science, Multidisciplinary)

We investigated a potential of femtosecond laser sintering of silicon carbide (SiC) using the nanoparticles in air. A SiC nanoparticle ink including polyvinylpyrrolidone and ethylene glycol exhibited intense absorption by SiC nanoparticles at the wavelength of 780 nm. The whole of the sintered film patterns from the surface to the bottom underwent significant oxidation at a scanning speed of 1 mm/s, suggesting that the excessive energy irradiation generated silicon oxides. In contrast, the patterns fabricated by laser scanning at a raster pitch of 30 $$mu$$m at which a sintered area was observed at a scanning speed of 5 mm/s, exhibited no significant difference in oxidation of the raw SiC nanoparticles except for the surfaces from 1.72 $$mu$$m. These results indicate that the irradiation of femtosecond laser pulses generated the sintered SiC patterns without additional atmospheric oxidation of the raw materials because of its low heat accumulation. In additions, the dispersant of polyvinylpyrrolidone and ethylene glycol did not affect the sintering by an X-ray photoelectron spectroscopy. This vacuum-free direct printing technique has the potential for additive manufacturing.

Journal Articles

Step unbunching phenomenon on 4H-SiC (0001) surface during hydrogen etching

Sakakibara, Ryotaro*; Bao, J.*; Yuhara, Keisuke*; Matsuda, Keita*; Terasawa, Tomoo; Kusunoki, Michiko*; Norimatsu, Wataru*

Applied Physics Letters, 123(3), p.031603_1 - 031603_4, 2023/07

 Times Cited Count:1 Percentile:54.89(Physics, Applied)

We here report a step unbunching phenomenon, which is the inverse of the phenomenon of step bunching. When a 4H-SiC (0001) surface is annealed at a high temperature, step bunching arises due to the different velocities of the step motion in adjacent steps, resulting in steps with a height of more than several nanometers. We found that the bunched steps, thus, obtained by hydrogen etching in an Ar/H$$_{2}$$ atmosphere were "unbunched" into lower height steps when annealed subsequently at lower temperatures. This unbunching phenomenon can be well explained by the consequence of the competition between energetics and kinetics. Our findings provide another approach for the surface smoothing of SiC by hydrogen etching and may give significant insight into the application of SiC power devices and two-dimensional materials growth techniques in general.

Journal Articles

The Development of a Multiphysics Coupled Solver for Studying the Effect of Dynamic Heterogeneous Configuration on Particulate Debris Bed Criticality and Cooling Characteristics

Li, C.-Y.; Wang, K.*; Uchibori, Akihiro; Okano, Yasushi; Pellegrini, M.*; Erkan, N.*; Takata, Takashi*; Okamoto, Koji*

Applied Sciences (Internet), 13(13), p.7705_1 - 7705_29, 2023/07

 Times Cited Count:1 Percentile:0(Chemistry, Multidisciplinary)

Journal Articles

Establishing an evaluation method for the aging phenomenon by physical force in fuel debris

Suzuki, Seiya; Arai, Yoichi; Okamura, Nobuo; Watanabe, Masayuki

Journal of Nuclear Science and Technology, 60(7), p.839 - 848, 2023/07

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The fuel debris, consisting of nuclear fuel materials and reactor structural materials, generated in the accident of Fukushima Daiichi Nuclear Power Plant can become deteriorated like rocks under the changes of environmental temperature. Although the fuel debris have been cooled by water for 10 years, they are affected by seasonal and/or day-and-night temperature changes. Therefore, in evaluating the aging behavior of the fuel debris, it is essential to consider the changes in environmental temperature. Assuming that the fuel debris are deteriorated, radioactive substances that have recently undergone micronization could be eluted into the cooling water, and such condition may affect defueling methods. We focused on the effect of repeated changes in environmental temperature on the occurrence of cracks, and an accelerated test using simulated fuel debris was carried out. The length of the crack increases with increasing number of heat cycle; therefore, the fuel debris become brittle by stress caused by thermal expansion and contraction. In conclusion, it was confirmed that the mechanical deterioration of the fuel debris is similar to that of rocks or minerals, and it became possible to predict changes in the length of the crack in the simulated fuel debris and environmental model.

Journal Articles

The Effects of unburned-gas temperature and pressure on the unstable behavior of cellular-flame fronts generated by intrinsic instability in hydrogen-air lean premixed flames under adiabatic and non-adiabatic conditions; Numerical simulation based on the detailed chemical reaction model

Thwe Thwe, A.; Kadowaki, Satoshi; Nagaishi, Ryuji

Journal of Nuclear Science and Technology, 60(6), p.731 - 742, 2023/06

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

In this study, we performed numerical calculations of unsteady reaction flow considering detailed chemical reactions, investigated the unstable behavior of hydrogen-air dilute premixed flame due to intrinsic instability, and clarified the effects of unburned gas temperature and pressure. I made it. The unstable behavior of the flame in a wide space was simulated, and the burning rate of the cellular flame was obtained. Then, the effects of heat loss and flame scale on flame unstable behavior were investigated. The burning velocity of a planar flame increases as the unburned-gas temperature increases and it decreases as the unburned-gas pressure and heat loss increase. The normalized burning velocity increases when the pressure increases and heat loss becomes large, and it decreases when the temperature increases. This is because the high unburned-gas pressure and heat loss promote the unstable behavior and instability of flame.

JAEA Reports

Development of thin SiC neutron detector with high radiation resistance (Contract research); FY2020 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Kyoto University*

JAEA-Review 2022-068, 90 Pages, 2023/05

JAEA-Review-2022-068.pdf:3.55MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2020. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2018, this report summarizes the research results of the "Development of thin SiC neutron detector with high radiation resistance" conducted from FY2018 to FY2021 (this contract was extended to FY2021). Since the final year of this proposal was FY2021, the results for four fiscal years were summarized. In the works for debris retrieval, it is required to install subcritical surveillance radiation monitors that can surely work for long time under extremely high gamma-ray radiation environment. However, there have been problems such as remote control of conventional neutron detectors is difficult because heavy radiation shields are needed.

Journal Articles

Research on improvement of HTGR core power-density, 4; Feasibility study for a reactor core

Okita, Shoichiro; Mizuta, Naoki; Takamatsu, Kuniyoshi; Goto, Minoru; Yoshida, Katsumi*; Nishimura, Yosuke*; Okamoto, Koji*

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 10 Pages, 2023/05

Journal Articles

Study on actinide burning core concepts for the future phaseout of a fast reactor fuel cycle

Mori, Tetsuya; Naganuma, Masayuki; Oki, Shigeo

Nuclear Technology, 209(4), p.532 - 548, 2023/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

This paper deals with a conceptual study on a plutonium (Pu) and minor actinide (MA) burning fast reactor core for the distant future phaseout of a fast-reactor fuel cycle after it is commercialized and used for a long time. This burning core aims to reduce the Pu and MA inventories contained in the fuel cycle through multiple recycling. A key point for the core design is the degradation of Pu and MA during multiple recycling. This degradation affects the core feasibility by increasing the sodium void reactivity and decreasing the absolute value of the Doppler constant. A feasible core concept was found by incorporating the following three factors to improve the reactivity coefficients: core flattening, fuel burnup reduction, and the use of silicon carbide (SiC) in the cladding and wrapper tubes. Notably, softening the neutron spectrum using the SiC structural material not only improved the reactivity coefficients but also indirectly mitigated the degradation of Pu and MA. Consequently, the designed core allowed for multiple recycling to continue until the Pu and MA reduced significantly, particularly by about 99% in a phaseout scenario starting from a fast-reactor fleet of 30-GWe nuclear power capacity. Fast reactors were found to have the potential to become self-contained energy systems that can minimize the inventories of Pu they produced themselves, as well as long-lived MA. Fast reactors can be among the important options for environmental burden reduction in the future.

JAEA Reports

Development of stable solidification technique of ALPS sediment wastes by apatite ceramics (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Tokyo Institute of Technology*

JAEA-Review 2022-076, 227 Pages, 2023/03

JAEA-Review-2022-076.pdf:9.42MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station (1F), Tokyo Electric Power Company Holdings, Inc. (TEPCO). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Development of stable solidification technique of ALPS sediment wastes by apatite ceramics" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. The present study aims to establish an apatite solidification process of radioactive sediment wastes, which were generated from the ALPS process manipulating the large amount of contaminated water from 1F. We selected the precipitation method and post stabilization for engineering-scale process. Investigation on composition, structure and elution properties of apatite and related phosphate waste forms fabricated from the simulated ALPS sediment wastes were implemented.

JAEA Reports

Estimation of the in-depth debris status of Fukushima Unit-2 and Unit-3 with Multi-physics modeling (Contract research); FY2021 Nuclear Energy Science & Technology and Human Resource Development Project

Collaborative Laboratories for Advanced Decommissioning Science; Waseda University*

JAEA-Review 2022-054, 150 Pages, 2023/02

JAEA-Review-2022-054.pdf:7.26MB

The Collaborative Laboratories for Advanced Decommissioning Science (CLADS), Japan Atomic Energy Agency (JAEA), had been conducting the Nuclear Energy Science & Technology and Human Resource Development Project (hereafter referred to "the Project") in FY2021. The Project aims to contribute to solving problems in the nuclear energy field represented by the decommissioning of the Fukushima Daiichi Nuclear Power Station, Tokyo Electric Power Company Holdings, Inc. (hereafter referred to "1F"). For this purpose, intelligence was collected from all over the world, and basic research and human resource development were promoted by closely integrating/collaborating knowledge and experiences in various fields beyond the barrier of conventional organizations and research fields. The sponsor of the Project was moved from the Ministry of Education, Culture, Sports, Science and Technology to JAEA since the newly adopted proposals in FY2018. On this occasion, JAEA constructed a new research system where JAEA-academia collaboration is reinforced and medium-to-long term research/development and human resource development contributing to the decommissioning are stably and consecutively implemented. Among the adopted proposals in FY2019, this report summarizes the research results of the "Estimation of the in-depth debris status of Fukushima Unit-2 and Unit-3 with multi-physics modeling" conducted from FY2019 to FY2021. Since the final year of this proposal was FY2021, the results for three fiscal years were summarized. Continuous update on understanding of the damaged 1F reactors is important for safe and efficient decommissioning of the reactors. This study aimed to estimate the in-depth debris status of the damaged 1F Unit-2 and Unit-3 through multi-physics modeling, which comprises of MPS method, simulated molten debris relocation experiment and high-temperature melt property data acquisition in the three-year project from FY2019.

Journal Articles

Semiconductor pulse power supplies for accelerators at J-PARC

Takayanagi, Tomohiro; Ono, Ayato; Fuwa, Yasuhiro; Shinozaki, Shinichi; Horino, Koki*; Ueno, Tomoaki*; Sugita, Moe; Yamamoto, Kazami; Oguri, Hidetomo; Kinsho, Michikazu; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.242 - 246, 2023/01

At J-PARC, semiconductor short pulse power supplies to replace kicker power supplies and semiconductor long pulse power supplies to replace klystron power supply systems are under construction. We have fabricated a 40kV/2kA/1.2$$mu$$s unit power supply that employs a linear transformer drivers (LTD) system for kickers. Currently, we are working on a high voltage insulating cylinder insulator that suppresses corona discharges using only the insulator structure, without using insulating oil. In addition, the MARX system was adopted for klystron power supply system. A main circuit unit for 8kV/60A/830$$mu$$s rectangular pulse output and an 800V/60A correction circuit unit that improves the flat top droop from 10% to 1% were manufactured. Furthermore, a 2.2kV/2.4kW high voltage SiC inverter charger has been fabricated for this MARX power supply. The presentation will report the evaluation results of each test and prospects for semiconductor pulse power supplies.

Journal Articles

Construction of low-jitter circuit for new kicker power supply using next-generation power semiconductor

Oda, Kodai; Takayanagi, Tomohiro; Ono, Ayato; Horino, Koki*; Ueno, Tomoaki*; Sugita, Moe; Morishita, Takatoshi; Iinuma, Hiromi*; Tokuchi, Akira*; Kamezaki, Hiroaki*; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.610 - 614, 2023/01

Kicker system is being used to kick the accelerated 3 GeV beam into the transport lines in RCS of J-PARC. The current kicker power supply applies thyratrons to discharge switches. We are developing a new kicker power supply using next-generation power semiconductors. The timing of the semiconductor switch operation is determined by the input of an external trigger signal. Large timing jitter causes unstable output pulses and beam loss due to beam orbit deviate from reference orbit. Therefore, a low jitter circuit that achieves high repeatability of 2 ns or less will be developed for the new kicker power supply. A prototype trigger generator has been fabricated, and jitter has been evaluated. The results of the evaluation test and the circuit configuration plan for reducing jitter will be reported.

Journal Articles

Instability phenomena of lean hydrogen/oxygen/inert-gas premixed flames on a flat burner

Katsumi, Toshiyuki; Thwe Thwe, A.; Kadowaki, Satoshi

Journal of Visualization, 25(5), p.1075 - 1083, 2022/10

 Times Cited Count:1 Percentile:20.8(Computer Science, Interdisciplinary Applications)

Lean combustion and inert-gas addition are useful to control the burning velocity of hydrogen premixed flames, and it is well known that the cellular structure forms on the front of lean hydrogen flames owing to intrinsic instability. However, the influences of inert-gas addition on the instability phenomena of lean hydrogen premixed flames are not understood fully, and then it is needed to be investigated the flame instability experimentally. In the experiments, the cellular structure and fluctuation of H$$_{2}$$/O$$_{2}$$/inert gases (Ar, N$$_{2}$$,CO$$_{2}$$) premixed flames on a flat burner were obtained using direct observation, laser diagnostics and light emission intensity to elucidate the characteristics of instability phenomena. As the results, the correlation of inert-gas addition, equivalence ratio and total flow rate with the characteristics of cellular flames was revealed, and the influences of these parameters on flame instability were discussed.

JAEA Reports

The Preliminary tests of the plasma melting treatment for homogenization of low-level radioactive wastes

Nakashio, Nobuyuki*; Osugi, Takeshi; Kurosawa, Shigenobu; Ishikawa, Joji; Hemmi, Ko; Iketani, Shotaro; Yokobori, Tomohiko

JAEA-Technology 2022-016, 47 Pages, 2022/08

JAEA-Technology-2022-016.pdf:2.23MB

The Nuclear Science Research Institute (NSRI) of the Japan Atomic Energy Agency (JAEA) started operation of the Advanced Volume Reduction Facilities (AVWF) for production of waste packages for disposal of low-level radioactive solid wastes (LLW). To clarify the operating conditions for homogenization of non-metallic LLW, preliminary tests were carried out using the plasma melting furnace of the non-metal melting unit. The fluidity of molten waste influences homogenization conditions of solidified products. It was clarified that the viscosity, which is determined by the chemical composition and the melting temperature, influence the fluidity of molten waste greatly through previous literature review and the small-scale melting tests. In the preliminary tests, the simulated waste with a cold tracer loaded in 200 L drums were melted. Using the waste chemical components (basicity, iron oxide concentration) as an experimental parameter, the homogeneity of the chemical components of the solidified product was investigated and the homogenization conditions of melting tests were examined. The retention ratio of the tracer in the molten bath was also confirmed. The viscosity of the molten wastes was measured and the correlation with homogeneity was examined. In addition, the technical requirements that should be concerned in advance for future actual operation were discussed.

Journal Articles

Nuclear data as foundation of nuclear research and development

Fukahori, Tokio; Nakayama, Shinsuke; Katabuchi, Tatsuya*; Shigyo, Nobuhiro*

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 64(7), p.413 - 414, 2022/07

The Investigation Advisory Committee on Nuclear Data monitors global nuclear research and development trends, and conducts collaborative nuclear data activities with domestic and foreign academic institutions in a wide range of fields. The aims are to contact, to exchange information, and to build an interdisciplinary cooperation system. Reported are the activities on the request list site, human resources development, and roadmap creation regarding nuclear data directly related to future nuclear data research activities, among the main activities in the 2019-2020 period.

Journal Articles

Impact of post-nitridation annealing in CO$$_{2}$$ ambient on threshold voltage stability in 4H-SiC metal-oxide-semiconductor field-effect transistors

Hosoi, Takuji*; Osako, Momoe*; Moges, K.*; Ito, Koji*; Kimoto, Tsunenobu*; Sometani, Mitsuru*; Okamoto, Mitsuo*; Yoshigoe, Akitaka; Shimura, Takayoshi*; Watanabe, Heiji*

Applied Physics Express, 15(6), p.061003_1 - 061003_5, 2022/06

 Times Cited Count:2 Percentile:34.67(Physics, Applied)

The combination of NO annealing and subsequent post-nitridation annealing (PNA) in CO$$_{2}$$ ambient for SiO$$_{2}$$/SiC structures has been demonstrated to be effective in obtaining both high channel mobility and superior threshold voltage stability in SiC-based metal-oxide-semiconductor field-effect transistors (MOSFETs). N atoms on the SiO$$_{2}$$ side of the SiO$$_{2}$$/SiC interface incorporated by NO annealing, which are plausible cause of charge trapping sites, could be selectively removed by CO$$_{2}$$-PNA at 1300$$^{circ}$$C without oxidizing the SiC. CO$$_{2}$$-PNA was also effective in compensating oxygen vacancies in SiO$$_{2}$$, resulting high immunity against both positive and negative bias-temperature stresses.

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